浏览全部资源
扫码关注微信
- About Journal
- Aims & scope
- Overview
- Indexing
- All issues
- Latest Issue
- Archive
- Online First
- Virtual Issues
- Authors
- Author’s Home
- Guide for Authors
- Copyright and License Term
- Peer Review
- Open access
- Ethics Policy
- Publication Agreement
Spatial distribution Characteristics of PAEs and key environmental factors in Yulin River in the Three Gorges Reservoir
- Journal of Civil and Environmental Engineering Vol. 44, Issue 6, Pages: 193-200(2022)
- 作者机构：
1.北京首创生态环保集团股份有限公司，北京 100044
2.首创爱华（天津）市政环境工程有限公司 天津 300060
3.重庆大学 三峡库区生态环境教育部重点实验室，重庆 400045
- 作者简介：
brief:WANG Ruilin (1988- ), main research interests: integrated water basin management and waste water treatment technology，E-mail: wz912076@qq.com.
LI Hong （corresponding author）， associate professor， doctorial supervisor， E-mail： hongli@cqu.edu.cn.
- 基金信息：National Natural Science Foundation of China(41877472)
DOI：10.11835/j.issn.2096-6717.2021.186
CLC： X522Received：06 August 2021，
Published：30 December 2022
- 稿件说明：
移动端阅览
王瑞霖,冉艳,黄维等.三峡库区御临河邻苯二甲酸酯类的空间分布特征及关键环境影响因子[J].土木与环境工程学报,2022,44(06):193-200.
WANG Ruilin,RAN Yan,HUANG Wei,et al.Spatial distribution Characteristics of PAEs and key environmental factors in Yulin River in the Three Gorges Reservoir[J].Journal of Civil and Environmental Engineering,2022,44(06):193-200.
王瑞霖,冉艳,黄维等.三峡库区御临河邻苯二甲酸酯类的空间分布特征及关键环境影响因子[J].土木与环境工程学报,2022,44(06):193-200. DOI： 10.11835/j.issn.2096-6717.2021.186.
WANG Ruilin,RAN Yan,HUANG Wei,et al.Spatial distribution Characteristics of PAEs and key environmental factors in Yulin River in the Three Gorges Reservoir[J].Journal of Civil and Environmental Engineering,2022,44(06):193-200. DOI： 10.11835/j.issn.2096-6717.2021.186.
摘要
为了解三峡库区内支流水体中邻苯二甲酸酯（PAEs）的来源、空间分布规律及影响其分布的主要环境因子，选取三峡库区库尾一级支流御临河上的5个断面：河口区、回水区（排花、舒家、梅溪）和不受三峡库区调度影响的上游来水区（东河）对PAEs进行了原位调研。基于皮尔逊相关性分析和主成分分析法确定御临河水体中6种PAEs的来源以及主要PAEs与环境因子的关系。结果表明：所监测断面中6种PAEs（DEP、DMP、DBP、BBP、DEHP和DnOP，US EPA）的总浓度为0.42~0.77 μg/L，5个监测断面PAEs平均总浓度依次为：河口（0.771 μg/L）>排花（0.638 μg/L）>梅溪（0.613 μg/L）>东河（0.566 μg/L）>舒家（0.421 μg/L）。通过对6种优先控制PAEs的解析发现，御临河水体中主要污染物为DBP、DMP和DEHP。皮尔逊相关性分析和主成分分析结果表明，DBP和DEHP显著正相关，可能与工农业生产活动及其过程中产生的“三废”有关；DMP和DEP具有中等强度的相关性，可能与当地居民的人为活动有关。
Abstract
In order to understand the source and spatial distribution regularities of PAEs and the main environmental factors affecting their distribution in the tributary of the Three Gorges Reservoir
Five sections in Yulin River
the first level tributa at the end of the Three Gorges Reservoir
were selected: the Estuary
the backwater area (Paihua
Shujia
Meixi) and the upsteam inflow area (Donghe)
which was not affected by the operation of the Three Gorges Reservoir
to conduct an in-situ investigation on PAEs. Based on Pearson correlation analysis and principal component analysis
the sources of six PAEs in Yulin River and the relationship between the main PAEs and environmental factors were identified. The results of in-situ investigations of 6 kinds of PAEs (DEP
DMP
DBP
BBP
DEHP and DnOP
according to US EPA) in five monitoring section of the Yulin River revealed that the total concentration of PAEs was in the range of 0.42~0.77 μg/L. The average total concentrations of PAEs in the five monitoring sections were: Estuary (0.771 μg/L) > Paihua (0.638 μg/L) > Meixi (0.613 μg/L) > Donghe (0.566 μg/L) > Shujia (0.421 μg/L)
with DMP
DBP and DEHP being the primary monomers. Based on the correlation analysis and principal component analysis
it was found that there was a significant positive correlation between DBP and DEHP
which may be related to industrial and agricultural production activities and the “three wastes” generated in the process. The moderate correlation between DMP and DEP indicated that these pollutants may be attributed from the anthropogenic activities of local residents.
关键词
Keywords
references
LIU Q , YANG H J , SHI Y X , et al . Research progress on phthalate esters (PAEs) organic pollutants in the environment [J]. Chinese Journal of Eco-Agriculture , 2012 , 20 ( 8 ): 968 - 975 .
张琳 . 袋装牛奶中邻苯二甲酸酯的检测及迁移规律研究 [D]. 河北 保定 : 河北农业大学 , 2013 .
ZHANG L . The determination and migration of phthalate ester in plastic bagged milk [D]. Baoding, Hebei : Hebei Agricultural University , 2013 . (in Chinese)
GIOVANOULIS G , BUI T , XU F C , et al . Multi-pathway human exposure assessment of phthalate esters and DINCH [J]. Environment International , 2018 , 112 : 115 - 126 .
SUN C Z , ZHANG G , ZHENG H , et al . Fate of four phthalate esters with presence of Karenia brevis: Uptake and biodegradation [J]. Aquatic Toxicology , 2019 , 206 : 81 - 90 .
WANIA F , MACKAY D . Tracking the distribution of persistent organic pollutants [J]. Environmental Science & Technology , 1996 , 30 ( 9 ): 390 - 396 .
SCHERINGER M , SALZMANN M , STROEBE M , et al . Long-range transport and global fractionation of POPs: Insights from multimedia modeling studies [J]. Environmental Pollution , 2004 , 128 ( 1/2 ): 177 - 188 .
CORSOLINI S , ADEMOLLO N , ROMEO T , et al . Persistent organic pollutants in edible fish: A human and environmental health problem [J]. Microchemical Journal , 2005 , 79 ( 1/2 ): 115 - 123 .
熊希瑶 , 贺聪聪 , 焦啸宇 , 等 . 水生态环境中邻苯二甲酸酯(PAEs)塑化剂的赋存及行为归趋 [J]. 中南民族大学学报(自然科学版) , 2021 , 40 ( 3 ): 238 - 245 .
XIONG X Y , HE C C , JIAO X Y , et al . Occurrence, behavior and fate of phthalate easters (PAEs) plasticizers in aquatic environmental systems [J]. Journal of South-Central University for Nationalities (Natural Science Edition) , 2021 , 40 ( 3 ): 238 - 245 . (in Chinese)
BENJAMIN S , MASAI E J , KAMIMURA N , et al . Phthalates impact human health: Epidemiological evidences and plausible mechanism of action [J]. Journal of Hazardous Materials , 2017 , 340 : 360 - 383 .
TRANFO G , PACI E , PIGINI D , et al . Phthalate metabolites in amniotic fluid and maternal urine samples [J]. Journal of Environmental Protection , 2014 , 5 ( 14 ): 1411 - 1418 .
ZHANG L L , LIU J L , LIU H Y , et al . The occurrence and ecological risk assessment of phthalate esters (PAEs) in urban aquatic environments of China [J]. Ecotoxicology , 2015 , 24 ( 5 ): 967 - 984 .
许川 , 舒为群 , 罗财红 , 等 . 三峡库区水环境多环芳烃和邻苯二甲酸酯类有机污染物健康风险评价 [J]. 环境科学研究 , 2007 , 20 ( 5 ): 57 - 60 .
XU C , SHU W Q , LUO C H , et al . Water environmental health risk assessment of PAHs and PAEs in the Three Gorges reservoir [J]. Research of Environmental Sciences , 2007 , 20 ( 5 ): 57 - 60 . (in Chinese)
HE M J , YANG T , YANG Z H , et al . Current state, distribution, and sources of phthalate esters and organophosphate esters in soils of the Three Gorges reservoir region, China [J]. Archives of Environmental Contamination and Toxicology , 2018 , 74 ( 3 ): 502 - 513 .
杨婷 , 何明靖 , 杨志豪 , 等 . 邻苯二甲酸酯在三峡库区消落带非淹水期土壤中污染特征及健康风险 [J]. 环境科学 , 2017 , 38 ( 10 ): 4187 - 4193 .
YANG T , HE M J , YANG Z H , et al . Occurrence, distribution and health risk of the phthalate esters in riparian soil in the fluctuating zone of the Three Gorges Reservoir [J]. Environmental Science , 2017 , 38 ( 10 ): 4187 - 4193 . (in Chinese)
LIN L , DONG L , MENG X Y , et al . Distribution and sources of polycyclic aromatic hydrocarbons and phthalic acid esters in water and surface sediment from the Three Gorges Reservoir [J]. Journal of Environmental Sciences , 2018 , 69 ( 7 ): 271 - 280 .
冉艳 , 何强 , 袁若愚 , 等 . 不同粒径悬移质泥沙对邻苯二甲酸二正丁酯的吸附特性 [J]. 土木与环境工程学报(中英文) , 2021 , 43 ( 5 ): 178 - 186 .
RAN Y , HE Q , YUAN R Y , et al . Adsorption characters of dibutyl phthalate in different grain-size suspended particulate matter [J]. Journal of Civil and Environmental Engineering , 2021 , 43 ( 5 ): 178 - 186 . (in Chinese)
HE Y , WANG Q M , HE W , et al . The occurrence, composition and partitioning of phthalate esters (PAEs) in the water-suspended particulate matter (SPM) system of Lake Chaohu, China [J]. Science of the Total Environment , 2019 , 661 : 285 - 293 .
杜娴 . 重庆主城两江水体与沉积物中邻苯二甲酸酯和多环芳烃污染水平及特征 [D]. 重庆 : 重庆大学 , 2012 .
DU X . Levels and characteristics of phthalate esters and polycyclic aromatic hydrocarbons in the Yangtze River and Jialing River from Chongqing’s urban areas [D]. Chongqing : Chongqing University , 2012 . (in Chinese)
吴亚非 , 李科 . 基于SPSS的主成分分析法在评价体系中的应用 [J]. 当代经济 , 2009 ( 3 ): 166 - 168 .
WU Y F , LI K . Application of SPSS based primary component analysis in comprehensive evaluation [J]. Contemporary Economics , 2009 ( 3 ): 166 - 168 . (in Chinese)
林莉 , 董磊 , 李青云 , 等 . 三峡库区水体和底泥中多环芳烃和邻苯二甲酸酯类分布和来源 [J]. 湖泊科学 , 2018 , 30 ( 3 ): 660 - 667 .
LIN L , DONG L , LI Q Y , et al . Distribution and sources of polycyclic aromatic hydrocarbons and phthalic acid esters in water and surface sediment from the Three Gorges Reservoir [J]. Journal of Lake Sciences , 2018 , 30 ( 3 ): 660 - 667 . (in Chinese)
沈思 , 王晓瑜 , 王海霞 , 等 . 细菌降解邻苯二甲酸酯的研究进展 [J]. 生物工程学报 , 2019 , 35 ( 11 ): 2104 - 2120 .
SHEN S , WANG X Y , WANG H X , et al . Advances in biodegradation of phthalates esters [J]. Chinese Journal of Biotechnology , 2019 , 35 ( 11 ): 2104 - 2120 . (in Chinese)
LI Y Y , HE W , LIU W X , et al . Impacts of anthropogenic activities on spatial variations of phthalate esters in water and suspended particulate matter from China’s lakes [J]. Science of the Total Environment ， 2020 , 724 : 138281 .
0
Views
5
下载量
2
CSCD
- L-PDFDownload
- WORDDownload
- Meta-XMLDownload
- BibTeXDownload
- EndnoteDownload
- RefMan Download
- NoteExpressDownload
- NoteFirstDownload
Publicity Resources
Related Articles
Related Author
Related Institution
AI问答- Address：Journals Department, Chongqing University, 174 Shazhengjie, Chongqing 400044, P.R.China Postal code：400044
- Tel：+86-23-65111322 Email：xuebao@cqu.edu.cn
- Technical support is provided by Beijing Founder electronics co., LTD 京ICP备09064830号-19
京公网安备11010802024621 - It is recommended to read the content of this site in Chrome&IE9+. Please switch to extreme mode in browser 360.
- Cookies We use cookies to help provide and enhance our service and tailor content. By continuing, you agree to the use of cookies.