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1.重庆大学 环境与生态学院,重庆 400045
2.重庆大学溧阳智慧城市研究院,江苏 溧阳 213300
3.溧阳市水利局,江苏 溧阳 213300
brief:ZHAI Jun (1977- ), professor, main research interests: theory and technology of wastewater treatment, E-mail: zhaijun@cqu.edu.cn.
Received:15 March 2022,
Published:25 August 2023
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ZHAI Jun, CHEN Rongrong, JIN Jing, et al. Research progress of aerobic granular sludge treatment of textile dyeing wastewater[J]. Journal of Civil and Environmental Engineering, 2023, 45(4): 182-191.
ZHAI Jun, CHEN Rongrong, JIN Jing, et al. Research progress of aerobic granular sludge treatment of textile dyeing wastewater[J]. Journal of Civil and Environmental Engineering, 2023, 45(4): 182-191. DOI: 10.11835/j.issn.2096-6717.2022.065.
纺织印染废水成分复杂,含有大量染料、重金属等有毒难降解污染物,是最难处理的工业废水之一。传统的生物处理法因耐毒性差、处理负荷低、受外部环境影响等存在一定的局限性,难以高效处理该类废水。好氧颗粒污泥胞外聚合物含量高,且含有大量氨基、羧基等官能团,此外,其具有不同的氧化还原微环境,能够有效吸附、降解污染物。但好氧颗粒污泥对印染废水中重金属的去除仍存在局限性,对染料的脱色和矿化效率仍有较大提升空间。针对纺织印染废水的污染物特性,总结并论述好氧颗粒污泥技术的优点及其对废水中重金属、偶氮染料的去除机理;综述好氧颗粒污泥处理模拟与实际纺织印染废水的研究进展,并对其运行方式进行总结分析。基于重金属离子去除存在局限性、染料降解不够彻底、实际废水具有复杂性等各种问题,展望其发展方向,以期为今后好氧颗粒污泥高效处理纺织印染废水的研究提供参考。
Textile dyeing wastewater is one of the most difficult industrial wastewaters to treat because it contains a large amount of toxic and refractory pollutants such as dyes
heavy metals. The traditional biological treatment process has certain limitations
such as poor toxicity resistance
low treatment load
and being affected by the external environment
making it difficult to efficiently treat this type of wastewater. Aerobic granular sludge (AGS) has a high content of extracellular polymeric substances and contains a large number of functional groups such as amino groups and carboxyl groups. In addition
it has different redox microenvironments
which can effectively adsorb and degrade pollutants. However
there are still limitations in the removal of heavy metals from printing and dyeing wastewater by AGS
and there is still much room for improvement in the decolorization and mineralization efficiency of dyes. According to the pollutant characteristics of textile dyeing wastewater
the advantages of AGS technology and the removal mechanism of heavy metals and azo dyes in wastewater are summarized and discussed. The research progress of AGS treatment simulated and actual textile dyeing wastewater is reviewed
and the operation mode is summarized and analyzed. Based on the limitations of heavy metal ion removal
insufficient dye degradation
and the complexity of actual wastewater
the development direction is prospected
in order to provide a reference for the future research on the efficient treatment of textile dyeing wastewater by AGS.
姜金宏 , 何席伟 , 熊晓敏 , 等 . 纺织印染废水毒性特征与控制技术研究进展 [J]. 工业水处理 , 2021 , 41 ( 6 ): 77 - 87 .
JIANG J H , HE X W , XIONG X M , et al . Research progress on toxicity characteristics and control technologies of textile dyeing wastewater [J]. Industrial Water Treatment , 2021 , 41 ( 6 ): 77 - 87 . (in Chinese)
YASEEN D A , SCHOLZ M . Textile dye wastewater characteristics and constituents of synthetic effluents: A critical review [J]. International Journal of Environmental Science and Technology , 2019 , 16 ( 2 ): 1193 - 1226 .
DENG D Y , LAMSSALI M , ARYAL N , et al . Textiles wastewater treatment technology: A review [J]. Water Environment Research , 2020 , 92 ( 10 ): 1805 - 1810 .
翟俊 , 柳沛松 , 赵聚姣 . 过一硫酸盐碱催化处理染料废水 [J]. 中国环境科学 , 2020 , 40 ( 2 ): 647 - 652 .
ZHAI J , LIU P S , ZHAO J J . Treatment of dye wastewater by base catalysis of peroxymonosulfate(PMS) [J]. China Environmental Science , 2020 , 40 ( 2 ): 647 - 652 . (in Chinese)
翟俊 , 徐长健 , 张子璇 , 等 . 含Cu 2+ 工业废水对Orbal氧化沟的冲击及调控 [J]. 中国给水排水 , 2016 , 32 ( 15 ): 37 - 41 .
ZHAI J , XU C J , ZHANG Z X , et al . Impact of industrial wastewater containing Cu 2+ on orbal oxidation ditch and its solutions [J]. China Water & Wastewater , 2016 , 32 ( 15 ): 37 - 41 . (in Chinese)
NANCHARAIAH Y V , KIRAN KUMAR REDDY G . Aerobic granular sludge technology: Mechanisms of granulation and biotechnological applications [J]. Bioresource Technology , 2018 , 247 : 1128 - 1143 .
YEMASHOVA N , KALYUZHNYI S . Microbial conversion of selected azo dyes and their breakdown products [J]. Water Science and Technology , 2006 , 53 ( 11 ): 163 - 171 .
TAY J H , IVANOV V , PAN S , et al . Specific layers in aerobically grown microbial granules [J]. Letters in Applied Microbiology , 2002 , 34 ( 4 ): 254 - 257 .
FRANCA R D G , PINHEIRO H M , LOURENÇO N D . Recent developments in textile wastewater biotreatment: Dye metabolite fate, aerobic granular sludge systems and engineered nanoparticles [J]. Reviews in Environmental Science and Bio/Technology , 2020 , 19 ( 1 ): 149 - 190 .
FRANCA R D G , OLIVEIRA M C , PINHEIRO H M , et al . Biodegradation products of a sulfonated azo dye in aerobic granular sludge sequencing batch reactors treating simulated textile wastewater [J]. ACS Sustainable Chemistry & Engineering , 2019 , 7 ( 17 ): 14697 - 14706 .
LIU Y R , LI K , XU W Y , et al . GO/PEDOT: NaPSS modified cathode as heterogeneous electro-Fenton pretreatment and subsequently aerobic granular sludge biological degradation for dye wastewater treatment [J]. Science of the Total Environment , 2020 , 700 : 134536 .
LIANG J Y , NING X N , SUN J , et al . Toxicity evaluation of textile dyeing effluent and its possible relationship with chemical oxygen demand [J]. Ecotoxicology and Environmental Safety , 2018 , 166 : 56 - 62 .
METHNENI N , MORALES-GONZÁLEZ J A , JAZIRI A , et al . Persistent organic and inorganic pollutants in the effluents from the textile dyeing industries: Ecotoxicology appraisal via a battery of biotests [J]. Environmental Research , 2021 , 196 : 110956 .
GITA S , SHUKLA S P , DESHMUKHE G , et al . Toxicity evaluation of six textile dyes on growth, metabolism and elemental composition (C, H, N, S) of microalgae spirulina platensis: The environmental consequences [J]. Bulletin of Environmental Contamination and Toxicology , 2021 , 106 ( 2 ): 302 - 309 .
VELUSAMY S , ROY A , SUNDARAM S , et al . A review on heavy metal ions and containing dyes removal through graphene oxide-based adsorption strategies for textile wastewater treatment [J]. Chemical Record , 2021 , 21 ( 7 ): 1570 - 1610 .
吴晓 , 崔建平 . UASB+生物接触氧化组合工艺处理纺织印染废水工程实例 [J]. 江西化工 , 2019 ( 4 ): 135 - 137 .
WU X , CUI J P . UASB + biological contact oxidation combined process to treat textile printing and dyeing wastewater engineering example [J]. Jiangxi Chemical Industry , 2019 ( 4 ): 135 - 137 . (in Chinese)
LOTITO A M , FRATINO U , MANCINI A , et al . Effective aerobic granular sludge treatment of a real dyeing textile wastewater [J]. International Biodeterioration & Biodegradation , 2012 , 69 : 62 - 68 .
YURTSEVER A , SAHINKAYA E , ÇINAR Ö . Performance and foulant characteristics of an anaerobic membrane bioreactor treating real textile wastewater [J]. Journal of Water Process Engineering , 2020 , 33 : 101088 .
苏辉 , 胡永贵 , 白茹 , 等 . 辫带式生物填料在纺织印染废水处理中的应用 [J]. 中国环保产业 , 2021 ( 3 ): 51 - 53 .
SU H , HU Y G , BAI R , et al . Application of braided biological fillers in textile printing and dyeing wastewater treatment [J]. China Environmental Protection Industry , 2021 ( 3 ): 51 - 53 . (in Chinese)
MALIK A , HUSSAIN M , UDDIN F , et al . Investigation of textile dyeing effluent using activated sludge system to assess the removal efficiency [J]. Water Environment Research , 2021 , 93 ( 12 ): 2931 - 2940 .
BEZERRA DE ARAUJO C M , FILIPE OLIVEIRA DO NASCIMENTO G , RODRIGUES BEZERRA DA COSTA G , et al . Adsorptive removal of dye from real textile wastewater using graphene oxide produced via modifications of hummers method [J]. Chemical Engineering Communications , 2019 , 206 ( 11 ): 1375 - 1387 .
PRIYA E S , SELVAN P S . Water hyacinth ( Eichhornia crassipes )- An efficient and economic adsorbent for textile effluent treatment - A review [J]. Arabian Journal of Chemistry , 2017 , 10 : S3548 - S3558 .
KIANI R , MIRZAEI F , GHANBARI F , et al . Real textile wastewater treatment by a sulfate radicals-Advanced Oxidation Process: Peroxydisulfate decomposition using copper oxide (CuO) supported onto activated carbon [J]. Journal of Water Process Engineering , 2020 , 38 : 101623 .
SHOUKAT R , KHAN S J , JAMAL Y . Hybrid anaerobic-aerobic biological treatment for real textile wastewater [J]. Journal of Water Process Engineering , 2019 , 29 : 100804 .
IMTIAZUDDIN S M , MUMTAZ M , MALLICK K A . Pollutants of wastewater characteristics in textile industries [J]. Journal of Basic & Applied Sciences , 2012 , 8 ( 2 ): 554 - 556 .
GURSOY-HAKSEVENLER B H , ATASOY-AYTIS E , DILAVER M , et al . Treatability of hazardous substances in industrial wastewater: Case studies for textile manufacturing and leather production sectors [J]. Environmental Monitoring and Assessment , 2022 , 194 ( 5 ): 1 - 19 .
AVLONITIS S A , POULIOS I , SOTIRIOU D , et al . Simulated cotton dye effluents treatment and reuse by nanofiltration [J]. Desalination , 2008 , 221 ( 1/2/3 ): 259 - 267 .
MAHMOUD D K , SALLEH M A M , KARIM W A , et al . Batch adsorption of basic dye using acid treated kenaf fibre char: Equilibrium, kinetic and thermodynamic studies [J]. Chemical Engineering Journal , 2012 , 181/182 : 449 - 457 .
HASSAN M M , CARR C M . Biomass-derived porous carbonaceous materials and their composites as adsorbents for cationic and anionic dyes: A review [J]. Chemosphere , 2021 , 265 : 129087 .
ARSLAN I , BALCIOGLU I A . Advanced oxidation of raw and biotreated textile industry wastewater with O 3 , H 2 O 2 /UV-C and their sequential application [J]. Journal of Chemical Technology & Biotechnology , 2001 , 76 ( 1 ): 53 - 60 .
PAŹDZIOR K , WRĘBIAK J , LEDAKOWICZ S . Treatment of industrial textile wastewater in biological aerated filters-microbial diversity analysis [J]. Fibres and Textiles in Eastern Europe , 2020 , 28 ( 1 ): 106 - 114 .
DHAOUEFI Z , TOLEDO-CERVANTES A , GHEDIRA K , et al . Decolorization and phytotoxicity reduction in an innovative anaerobic/aerobic photobioreactor treating textile wastewater [J]. Chemosphere , 2019 , 234 : 356 - 364 .
KHANDARE R V , GOVINDWAR S P . Phytoremediation of textile dyes and effluents: Current scenario and future prospects [J]. Biotechnology Advances , 2015 , 33 ( 8 ): 1697 - 1714 .
MORGENROTH E , SHERDEN T , VAN LOOSDRECHT M C M , et al . Aerobic granular sludge in a sequencing batch reactor [J]. Water Research , 1997 , 31 ( 12 ): 3191 - 3194 .
陈颖 , 陈垚 , 李聪 , 等 . 好氧颗粒污泥结构特点及稳定性研究进展 [J]. 工业水处理 , 2021 , 41 ( 10 ): 28 - 35 .
CHEN Y , CHEN Y , LI C , et al . Research progress on the structural characteristics and stability of aerobic granular sludge [J]. Industrial Water Treatment , 2021 , 41 ( 10 ): 28 - 35 . (in Chinese)
SARMA S , TAY J . Aerobic granulation for future wastewater treatment technology: Challenges ahead [J]. Environmental Science: Water Research & Technology , 2018 , 4 ( 1 ): 9 - 15 .
MASZENAN A M , LIU Y , NG W J . Bioremediation of wastewaters with recalcitrant organic compounds and metals by aerobic granules [J]. Biotechnology Advances , 2011 , 29 ( 1 ): 111 - 123 .
CAI F R , LEI L R , LI Y M , et al . A review of aerobic granular sludge (AGS) treating recalcitrant wastewater: Refractory organics removal mechanism, application and prospect [J]. Science of the Total Environment , 2021 , 782 : 146852 .
王磊 , 汪文东 , 刘懂 , 等 . 象山港流域入湾河流水体中重金属风险评价及其来源解析 [J]. 环境科学 , 2020 , 41 ( 7 ): 3194 - 3203 .
WANG L , WANG W D , LIU D , et al . Risk assessment and source analysis of heavy metals in the river of a typical bay watershed [J]. Environmental Science , 2020 , 41 ( 7 ): 3194 - 3203 . (in Chinese)
WANG L , LIU X , LEE D J , et al . Recent advances on biosorption by aerobic granular sludge [J]. Journal of Hazardous Materials , 2018 , 357 : 253 - 270 .
SAJJAD M , AZIZ A , KIM K S . Biosorption and binding mechanisms of Ni 2+ and Cd 2+ with aerobic granules cultivated in different synthetic media [J]. Chemical Engineering & Technology , 2017 , 40 ( 12 ): 2179 - 2187 .
GAI L H , WANG S G , GONG W X , et al . Influence of pH and ionic strength on Cu(Ⅱ) biosorption by aerobic granular sludge and biosorption mechanism [J]. Journal of Chemical Technology & Biotechnology , 2008 , 83 ( 6 ): 806 - 813 .
WANG L , WANG Y Y , LIU X , et al . A comprehensive comparison of bacterial and fungal aerobic granules: Formation, properties, surface modification, and biosorption of metals [J]. RSC Advances , 2015 , 5 ( 126 ): 104062 - 104070 .
SUN X F , MA Y , LIU X W , et al . Sorption and detoxification of chromium ( Ⅵ) by aerobic granules functionalized with polyethylenimine [J]. Water Research , 2010 , 44 ( 8 ): 2517 - 2524 .
马岩 . 高浓度偶氮染料废水处理技术的研究 [D]. 天津 : 天津大学 , 2008 .
MA Y . Study on high concentration azo dye waste water treatment technology [D]. Tianjin : Tianjin University , 2008 . (in Chinese)
顾平 , 刘奎 , 杨造燕 . Fenton 试剂处理活性黑 KBR 染料废水研究 [J]. 中国给水排水 , 1997 , 13 ( 6 ): 16 - 18 .
GU P , LIU K , YANG Z Y . A study on treatment of active black KBR dyestuff wastewater by Fenton reagent [J]. China Water & Wastewater , 1997 , 13 ( 6 ): 16 - 18 . (in Chinese)
LOURENÇO N D , FRANCA R D G , MOREIRA M A , et al . Comparing aerobic granular sludge and flocculent sequencing batch reactor technologies for textile wastewater treatment [J]. Biochemical Engineering Journal , 2015 , 104 : 57 - 63 .
HISAINDEE S , MEETANI M A , RAUF M A . Application of LC-MS to the analysis of advanced oxidation process (AOP) degradation of dye products and reaction mechanisms [J]. TrAC Trends in Analytical Chemistry , 2013 , 49 : 31 - 44 .
SHAH M . Effect of anaerobic granular sludge in degradation of two azo dyes [J]. International Journal of Environmental Research , 2015 , 9 : 1351 - 1356 .
郭亚平 , 方继前 , 谢练武 , 等 . 污泥细菌偶氮呼吸机制与偶氮染料降解矿化机理 [J]. 环境工程 , 2012 , 30 ( Sup 2 ): 32 - 35 .
GUO Y P , FANG J Q , XIE L W , et al . Review on azorespiration, biodegradation and mineralization mechanisms of azo dyes related to sludge bacteria [J]. Environmental Engineering , 2012 , 30 ( Sup2 ): 32 - 35 . (in Chinese)
MANAVI N , KAZEMI A S , BONAKDARPOUR B . The development of aerobic granules from conventional activated sludge under anaerobic-aerobic cycles and their adaptation for treatment of dyeing wastewater [J]. Chemical Engineering Journal , 2017 , 312 : 375 - 384 .
YAN L K Q , FUNG K Y , NG K M . Aerobic sludge granulation for simultaneous anaerobic decolorization and aerobic aromatic amines mineralization for azo dye wastewater treatment [J]. Environmental Technology , 2018 , 39 ( 11 ): 1368 - 1375 .
FATIMA M , SAEED M , ASLAM M , et al . Application of novel bacterial consortium for biodegradation of aromatic amine 2-ABS using response surface methodology [J]. Journal of Microbiological Methods , 2020 , 174 : 105941 .
VALLI NACHIYAR C , SUSEELA RAJAKUMAR G . Biodegradation of 8-anilino-1-naphthalenesulfonic acid by pseudomonas aeruginosa [J]. Journal of Industrial Microbiology & Biotechnology , 2006 , 33 ( 10 ): 845 - 849 .
BIALA S , CHADHA P , SAINI H S . Biodegradation of 4-aminobenzenesulfonate by indigenous isolate Shinella yambaruensis SA1 and its validation by genotoxic analysis [J]. Biotechnology and Bioprocess Engineering , 2014 , 19 ( 6 ): 1034 - 1041 .
JONSTRUP M , KUMAR N , MURTO M , et al . Sequential anaerobic-aerobic treatment of azo dyes: Decolourisation and amine degradability [J]. Desalination , 2011 , 280 ( 1/2/3 ): 339 - 346 .
FRANCA R D G , ORTIGUEIRA J , PINHEIRO H M , et al . Effect of SBR feeding strategy and feed composition on the stability of aerobic granular sludge in the treatment of a simulated textile wastewater [J]. Water Science and Technology , 2017 , 76 ( 5/6 ): 1188 - 1195 .
MATA A M T , PINHEIRO H M , LOURENÇO N D . Effect of sequencing batch cycle strategy on the treatment of a simulated textile wastewater with aerobic granular sludge [J]. Biochemical Engineering Journal , 2015 , 104 : 106 - 114 .
李黔花 , 李志华 , 岳秀 , 等 . 好氧颗粒污泥处理印染废水的效能及其微生物特征 [J]. 工业水处理 , 2020 , 40 ( 3 ): 43 - 48 .
LI Q H , LI Z H , YUE X , et al . Efficiency and microbial characteristics of aerobic granular sludge for textile dyeing wastewater treatment [J]. Industrial Water Treatment , 2020 , 40 ( 3 ): 43 - 48 . (in Chinese)
田沙沙 . Fenton-好氧颗粒污泥处理模拟染料废水研究 [D]. 武汉 : 华中科技大学 , 2011 .
TIAN S S . Treatment of simulated dye wastewater by Fenton-aerobic granular sludge process [D]. Wuhan : Huazhong University of Science and Technology , 2011 . (in Chinese)
MOGHADDAM S S , MOGHADDAM M R A . Aerobic granular sludge for dye biodegradation in a sequencing batch reactor with anaerobic/aerobic cycles [J]. Clean - Soil, Air, Water , 2016 , 44 ( 4 ): 438 - 443 .
FRANCA R D G , VIEIRA A , MATA A M T , et al . Effect of an azo dye on the performance of an aerobic granular sludge sequencing batch reactor treating a simulated textile wastewater [J]. Water Research , 2015 , 85 : 327 - 336 .
李黔花 . 好氧颗粒污泥处理印染废水的实验研究 [D]. 西安 : 西安建筑科技大学 , 2019 .
LI Q H . Experimental study on treatment of textile dyeing wastewater by aerobic granular sludge [D]. Xi,an: Xi,an University of Architecture and Technology , 2019 . (in Chinese)
赵哲 . 厌氧-A/O工艺处理印染废水参数研究及工程设计 [D]. 北京 : 北京林业大学 , 2020 .
ZHAO Z . Study on parameters and engineering design of printing and dyeing wastewater treatment by anaerobic-A/O process [D]. Beijing : Beijing Forestry University , 2020 . (in Chinese)
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